Nature Communications, Published online: 16 September 2026; doi:10.1038/s41467-026-77227-3 Precise twist-angle control in van der Waals (vdW) moiré superlattices enables the observation of emerging physical properties. Here, the authors demonstrate a reversible pressure-controlled rotational response in multilayer spiral WS2, corresponding to an effective average interlayer twist of 0.2° per layer.