Abstract Herein, we explore selectivity toward generation of ClOx (x=1-4) anions and durability of commercial polycrystalline free-standing boron-doped diamond (BDD) electrodes in synthetic ASTM seawater oxidation. 10 min electrooxidation experiments at current densities from 1 to 100 mA/cm2 revealed formation of ClO-, ClO3-, and ClO4- anions. ClO- anions were found to be the dominant reaction product, with concentrations exceeding those of ClO3- and ClO4- by two and five orders of magnitude, respectively. The same trend was observed in 0.5M NaCl at pH 8.2 that was used as a reference, although the ClO3- concentration was found to be ca 30% higher. ClO- ions were generated in seawater with ca 85% Faradaic efficiency (FE), which was lower than that in 0.5M NaCl. This difference was attributed to parasitic reactions of ClO- with trace elements and organic impurities present in seawater. We demonstrated that radical scavengers such as H3BO3 and HCO3- present in seawater do not affect FEs of the ClO- production. 
 The 48 h durability tests demonstrated a slight performance decay, more pronounced in seawater. Performance decay was accompanied by the BDD surface oxidation with formation of carbonyl, carboxyl and hydroxyl groups, dominated by OH groups. 
Seawater Oxidation on Boron-Doped Diamond Electrodes
Olga Baturina·Andrew P. Purdy·Rachel Nixon·Christopher Katilie·Bradford B. Pate·Dagmar H. Leary·Graham T. Cheek

