The direct recycling of spent cathode materials is a promising strategy for a sustainable supply chain but remains challenging for industrial-sourced cathode black mass due to its complex morphology and heterogeneous impurities. Here, we report an all‑dry and scalable process that directly regenerates spent LiNi0.5Co0.2Mn0.3O2 (NCM523) black mass into high‑performance cathode materials. By integrating plasma-assisted mechanochemistry with thermal annea