Single-Metal-Anchored 1D Mesoporous Channels to Enable Accelerated Redox Kinetics for Lithium-Sulfur Batteries
Dequn Zhao·Wenhuan Huang·Yanan Zhang·Xingxing Zhang·Xuehan Hou·Hong Wang·Xiangyu Liu·Feiyang Yin·Wei Zhou·Shun Wang
Abstract Metal–organic frameworks (MOFs) have been demonstrated as promising separators for lithium-sulfur batteries (LSBs) owing to their highly tunable porous structures and intrinsic metal sites, which can guide uniform Li + deposition, catalyze polysulfide conversion, and suppress polysulfide shuttling. However, conventional MOFs often have insufficient catalytic activity and Li + transport control, and the role of their internal pore structure in regulating Li + flux and polysulfide convers